Show simple item record

dc.contributor.authorGao, Shilunen_US
dc.contributor.authorCannon, Andrewen_US
dc.contributor.authorSun, Feiyuanen_US
dc.contributor.authorPan, Yiyangen_US
dc.contributor.authorYang, Dandanen_US
dc.contributor.authorGe, Siruien_US
dc.contributor.authorLiu, Nianen_US
dc.contributor.authorSokolov, Alexei P.en_US
dc.contributor.authorRyan, Emilyen_US
dc.contributor.authorYang, Huabinen_US
dc.contributor.authorCao, Peng-Feien_US
dc.date.accessioned2022-05-11T19:37:57Z
dc.date.available2022-05-11T19:37:57Z
dc.date.issued2021-08
dc.identifier.citationS. Gao, A. Cannon, F. Sun, Y. Pan, D. Yang, S. Ge, N. Liu, A.P. Sokolov, E. Ryan, H. Yang, P.-.F. Cao. 2021. "Glass-fiber-reinforced polymeric film as an efficient protecting layer for stable Li metal electrodes." Cell Reports Physical Science, Volume 2, Issue 8, 100534. https://doi.org/10.1016/j.xcrp.2021.100534
dc.identifier.issn2666-3864
dc.identifier.urihttps://hdl.handle.net/2144/44397
dc.description.abstract[SUMMARY] With numerous reports on protecting films for stable lithium (Li) metal electrodes, the key attributes for how to construct these efficient layers have rarely been fully investigated. Here, we report a rationally designed hybrid protective layer (HPL) with each component aligning with one key attribute; i.e., cross-linked poly(dimethylsiloxane) (PDMS) enhances flexibility, polyethylene glycol (PEG) provides homogeneous ion-conducting channels, and glass fiber (GF) affords mechanical robustness. A significant improvement of the electrochemical performance of HPL-modified electrodes can be achieved in Li/HPL@Cu half cells, HPL@Li/HPL@Li symmetric cells, and HPL@Li/LiFePO4 full cells. Even with an industrial standard LiFePO4 cathode (96.8 wt % active material), the assembled cell still exhibits a capacity retention of 90% after 100 cycles at 1 C. More importantly, the functionality of each component has been studied comprehensively via electrochemical and physical experiments and simulations, which will provide useful guidance on how to construct efficient protective layers for next-generation energy storage devices.en_US
dc.languageen
dc.language.isoen_US
dc.publisherElsevier BVen_US
dc.relation.ispartofCell Reports Physical Science
dc.rightsCopyright 2021 The Authors. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).en_US
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/4.0/
dc.titleGlass-fiber-reinforced polymeric film as an efficient protecting layer for stable Li metal electrodesen_US
dc.typeArticleen_US
dc.description.versionPublished versionen_US
dc.identifier.doi10.1016/j.xcrp.2021.100534
pubs.elements-sourcecrossrefen_US
pubs.organisational-groupBoston Universityen_US
pubs.organisational-groupBoston University, College of Engineeringen_US
pubs.organisational-groupBoston University, College of Engineering, Department of Mechanical Engineeringen_US
pubs.publication-statusPublisheden_US
dc.identifier.mycv715725


This item appears in the following Collection(s)

Show simple item record

Copyright 2021 The Authors. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
Except where otherwise noted, this item's license is described as Copyright 2021 The Authors. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).